The Synergistic Effect of NaHSO4 and NaCl Salts on Corrosion Inhibition Performance of Two Gemini Cationic Surfactant Ionic Liquids
E. Kowsari （ Department of Chemistry, Amirkabir University of Technology, No. 424, Hafez Avenue, 1591634311, Tehran, Iran. ）
M. Payami （ Department of Chemistry, Amirkabir University of Technology, No. 424, Hafez Avenue, 1591634311, Tehran, Iran. ）
E. Kamali Ardakani （ Department of Chemistry, Amirkabir University of Technology, No. 424, Hafez Avenue, 1591634311, Tehran, Iran. ）
S. Kholghi Eshkalak （ b Department of Polymer Engineering and Color Technology, Amirkabir University of Technology, 424 Hafez Ave, 15875-4413, Tehran, Iran. c Department of Mechanical Engineering, Center for Nanofibers & Nanotechnology, Faculty of Engineering, National University of Singapore, Singapore 117576 ）
M. Ghambarian （ Gas Conversion Department, Faculty of Petrochemicals, Iran Polymer and Petrochemical Institute, P.O. Box 14975-112, Tehran, Iran ）
R. Amini （ Department of surface coating and Corrosion, Institute for Color Science and Technology (ICST), PO 16765-654, Tehran, Iran ）
B. Ramezanzadeh （ Gas Conversion Department, Faculty of Petrochemicals, Iran Polymer and Petrochemical Institute, P.O. Box 14975-112, Tehran, Iran ）
A Ehsani （ Department of Chemistry, Faculty of Science, University of Qom, Alghadir Blvd., Qom 3716146611, Iran ）
S. Ramakrishna
https://doi.org/10.37155/2717-526X-0201-4Abstract
In this study, two imidazolium-based ionic liquid surfactants (TSIL and EFAIL) were first synthesized, and then investigated the synergistic effects of NaHSO4 and NaCl salts on corrosion inhibition performance of TSIL and EFAIL inhibitors on low carbon steel samples in 1M HCl solution. For this aim, the electrochemical techniques of potentiodynamic polarization and electrochemical impedance spectroscopy (EIS), surface morphology analyses, and quantum chemical calculations were employed. Results showed that adding salts to acidic solutions containing EFAIL and TSIL increased their inhibition efficiency. Furthermore, addition of NaHSO4 to TSIL-containing solution could further increase the inhibition efficiency compared to other mixtures of the salts and the inhibitors. The DFT results also revealed that the energy gap of TSIL is lower than that of EFAIL, implying that TSIL has more chemical reactivity and less kinetic stability than EFAIL.
Keywords
Ionic liquid surfactant; EIS; polarization; acid corrosion; surface tension; density functional theoryFull Text
PDFReferences
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[14] F. Bentiss, C. Jama, B. Mernari, H. El Attari, L. El Kadi, M. Lebrini, M. Traisnel, M. Lagrenée, Corrosion control of mild steel using 3,5-bis(4-methoxyphenyl)-4-amino-1,2,4-triazole in normal hydrochloric acid medium, Corros. Sci. 51 (2009) 1628–1635.
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[16] X.G. Li, M.R. Huang, J.F. Zeng, M.F. Zhu, The preparation of polyaniline waterborne latex nanoparticles and their films with anti-corrosivity and semi-conductivity, Colloids Surfaces A Physicochem. Eng. Asp. 248 (2004) 111–120.
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[21] M.H. Wang, Y.J. Li, Z.X. Xie, C. Liu, E.S. Yeung, Fabrication of large-scale one-dimensional Au nanochain and nanowire networks by interfacial self-assembly, Mater. Chem. Phys. 119 (2010) 153–157.
[22] B. Dong, X. Zhao, L. Zheng, J. Zhang, N. Li, T. Inoue, Aggregation behavior of long-chain imidazolium ionic liquids in aqueous solution: Micellization and characterization of micelle microenvironment, Colloids Surfaces A Physicochem. Eng. Asp. 317 (2008) 666–672.
[23] M. Corrales-Luna, T. Le Manh, M. Romero-Romo, M. Palomar-Pardavé, E.M. Arce-Estrada, 1-Ethyl 3-methylimidazolium thiocyanate ionic liquid as corrosion inhibitor of API 5L X52 steel in H 2 SO 4 and HCl media, Corros. Sci. 153 (2019) 85–99.
[24] S. Cao, D. Liu, H. Ding, J. Wang, H. Lu, J. Gui, Task-specific ionic liquids as corrosion inhibitors on carbon steel in 0.5 M HCl solution: An experimental and theoretical study, Corros. Sci. 153 (2019) 301–313.
[25] E. Kamali Ardakani, E. Kowsari, A. Ehsani, Imidazolium-derived polymeric ionic liquid as a green inhibitor for corrosion inhibition of mild steel in 1.0 M HCl: Experimental and computational study, Colloids Surfaces A Physicochem. Eng. Asp. (2019) 124195.
[26] N. V. Likhanova, M.A. Domínguez-Aguilar, O. Olivares-Xometl, N. Nava-Entzana, E. Arce, H. Dorantes, The effect of ionic liquids with imidazolium and pyridinium cations on the corrosion inhibition of mild steel in acidic environment, Corros. Sci. 52 (2010) 2088–2097.
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[28] L. Feng, S. Zhang, Y. Lu, B. Tan, S. Chen, L. Guo, Synergistic corrosion inhibition effect of thiazolyl-based ionic liquids between anions and cations for copper in HCl solution, Appl. Surf. Sci. 483 (2019) 901–911.
[29] X. Li, S. Deng, H. Fu, G. Mu, Inhibition effect of 6-benzylaminopurine on the corrosion of cold rolled steel in H2SO4 solution, Corros. Sci. 51 (2009) 620–634.
[30] G.N. Mu, X. Li, F. Li, Synergistic inhibition between o-phenanthroline and chloride ion on cold rolled steel corrosion in phosphoric acid, Mater. Chem. Phys. 86 (2004) 59–68.
[31] X. Li, L. Tang, L. Li, G. Mu, G. Liu, Synergistic inhibition between o-phenanthroline and chloride ion for steel corrosion in sulphuric acid, Corros. Sci. 48 (2006) 308–321.
[32] G.K. Gomma, Corrosion of low-carbon steel in sulphuric acid solution in presence of pyrazole-halides mixture, Mater. Chem. Phys. 55 (1998) 241–246.
[33] P.C. Okafor, Y. Zheng, Synergistic inhibition behaviour of methylbenzyl quaternary imidazoline derivative and iodide ions on mild steel in H2SO4 solutions, Corros. Sci. 51 (2009) 850–859.
[34] A.M. Ridhwan, A.A. Rahim, A.M. Shah, Synergistic effect of halide ions on the corrosion inhibition of mild steel in hydrochloric acid using mangrove tannin, Int. J. Electrochem. Sci. 7 (2012) 8091–8104.
[35] M.R. Adam, A.A. Rahim, A.M. Shah, Synergy between iodide ions and mangrove tannins as inhibitors of mild steel corrosion, Ann. For. Sci. 72 (2015) 9–15.
[36] M. Abdallah, S.T. Atwa, M.M. Salem, A.S. Fouda, Synergistic effect of some halide ions on the inhibition of zinc corrosion in hydrocchloric acid by tetrahydro carbazole derivatives compounds, Int. J. Electrochem. Sci. 8 (2013) 10001–10021.
[37] A.A. Farag, M.A. Hegazy, Synergistic inhibition effect of potassium iodide and novel Schiff bases on X65 steel corrosion in 0.5M H2SO4, Corros. Sci. 74 (2013) 168–177.
[38] M.M. Solomon, S.A. Umoren, M.A. Quraishi, M.A. Jafar Mazumder, Corrosion inhibition of N80 steel in simulated acidizing environment by N-(2-(2-pentadecyl-4,5-dihydro-1H-imidazol-1-YL) ethyl) palmitamide, J. Mol. Liq. 273 (2019) 476–487.
[39] G. Cui, J. Guo, Y. Zhang, Q. Zhao, S. Fu, T. Han, S. Zhang, Chitosan oligosaccharide derivatives as green corrosion inhibitors for P110 steel in a carbon-dioxide-saturated chloride solution, Carbohydr. Polym. 203 (2019) 386–395.
[40] H. Tian, W. Li, A. Liu, X. Gao, P. Han, R. Ding, C. Yang, D. Wang, Controlled delivery of multi-substituted triazole by metal-organic framework for efficient inhibition of mild steel corrosion in neutral chloride solution, Corros. Sci. 131 (2018) 1–16.
[41] J. Aljourani, K. Raeissi, M.A. Golozar, Benzimidazole and its derivatives as corrosion inhibitors for mild steel in 1M HCl solution, Corros. Sci. 51 (2009) 1836–1843.
[42] N. V Likhanova, P. Arellanes-Lozada, O. Olivares-Xometl, I. V Lijanova, J. Arriola-Morales, J. Carlos Mendoza-Hernandez, G. Corro, Ionic liquids with carboxylic-acid-derived anions evaluated as corrosion inhibitors under dynamic conditions, Int. J. Electrochem. Sci. 14 (2019) 2655–2671.
[43] A. Döner, R. Solmaz, M. Özcan, G. Kardas, G. Kardaş, Experimental and theoretical studies of thiazoles as corrosion inhibitors for mild steel in sulphuric acid solution, Corros. Sci. 53 (2011) 2902–2913.
[44] B.P. Markhali, R. Naderi, M. Mahdavian, M. Sayebani, S.Y. Arman, Electrochemical impedance spectroscopy and electrochemical noise measurements as tools to evaluate corrosion inhibition of azole compounds on stainless steel in acidic media, Corros. Sci. 75 (2013) 269–279.
[45] W. Li, A. Liu, H. Tian, D. Wang, Controlled Release of Nitrate and Molybdate Intercalated in Zn-Al-Layered Double Hydroxide Nanocontainers towards Marine Anticorrosion Applications, Colloid Interface Sci. Commun. 24 (2018) 18–23.
[46] J. Du, Y. Liu, P. Liu, Y. Liu, S. Gao, L. Zhang, Effect of Inhibitor based on Emulsion on Mild Steel Corrosion in Acid Environment, Int. J. Electrochem. Sci. 14 (2019) 4532–4545.
[47] R. Fuchs-Godec, M.G. Pavlović, Synergistic effect between non-ionic surfactant and halide ions in the forms of inorganic or organic salts for the corrosion inhibition of stainless-steel X4Cr13 in sulphuric acid, Corros. Sci. 58 (2012) 192–201.
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Copyright © 2020 E. Kowsari, saeideh kholghi eshkalak, M. Payami, E. Kamali Ardakani, S. Kholghi Eshkalak, M. Ghambarian, R. Amini, B. Ramezanzadeh, A Ehsani
Publishing time:2020-06-30
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